Ultrafast Terahertz Self-Induced Absorption and Phase Modulation on a Graphene-Based Thin Film Absorber

Graphene THz self-induced modulation

We demonstrate a thin film graphene-based THz perfect absorbing device whose absorption and phase characteristics can be modulated through THz self-actions in the sub-picosecond time scale. The device consists of a single-layer graphene placed on an ionic liquid substrate, back-plated by a metallic back-reflector, with the graphene doping level mediated through electrostatic gating. We experimentally record an absorption modulation of more than 3 orders of magnitude from the initial perfect absorption state, when the device is illuminated with THz field strengths in the range of 102 to 654 kV/cm. Furthermore, an absolute phase modulation of 130° is recorded. Detailed theoretical analysis indicates that the origin of the THz nonlinear response is the THz-induced heating of the graphene’s carriers that leads to a reduction of its conductivity and, consequently, to reduced absorption of the THz radiation. Our analysis also maps the temporal dynamics of the THz-induced temperature elevation of the graphene’s carriers, illustrating the ultrafast, sub-picosecond nature of the overall process. These results can find applications in future dynamically controlled flat optics and spatiotemporal shaping of intense THz electric fields.

Anastasios D. Koulouklidis, Anna C. Tasolamprou, Spyros Doukas, Eudokia Kyriakou, M. Said Ergoktas, Christina Daskalaki, Eleftherios N. Economou, Coskun Kocabas, Elefterios Lidorikis, Maria Kafesaki, and Stelios Tzortzakis, ACS Photonics 2022 9 (9), 3075-3082, DOI: 10.1021/acsphotonics.2c00828

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